Selective Hydrodeoxygenation of Biomass‐Derived Oxygenates to Unsaturated Hydrocarbons using Molybdenum Carbide Catalysts
ChemSusChem2013Vol. 6(5), pp. 798–801
Citations Over TimeTop 1% of 2013 papers
Hui Ren, Weiting Yu, M. Salciccioli, Ying Chen, Yulin Huang, Ke Xiong, Dionisios G. Vlachos, Jingguang G. Chen
Abstract
Which cleavage do you prefer? With a combination of density functional theory (DFT) calculations, surface science studies, and reactor evaluations, Mo(2)C is identified as a highly selective HDO catalyst to selectively convert biomass-derived oxygenates to unsaturated hydrocarbons through selective C-O bond scissions without C-C bond cleavage. This provides high-value HDO products for utilization as feedstocks for chemicals and fuels; this also reduces the overall consumption of H2 .
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