The Water/Methanol Complexation Induced Reentrant Coil-to-Globule-to-Coil Transition of Individual Homopolymer Chains in Extremely Dilute Solution
Journal of the American Chemical Society2001Vol. 123(7), pp. 1376–1380
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Abstract
Narrowly distributed ultralong linear poly(N-isopropylacrylamide) (PNIPAM) (Mw = 2.63 × 107 g/mol and Mw/Mn 50 mol %, m/n becomes 1. In the range of ∼17 mol % < xmethanol < 50 mol %, different intermediates with 1 ≤ m/n ≤ 5 coexist. The speculated structures of these complexes could be related to a water pentamer.
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