Molecular-Based Electronically Switchable Tunnel Junction Devices
Journal of the American Chemical Society2001Vol. 123(50), pp. 12632–12641
Citations Over TimeTop 1% of 2001 papers
C. Patrick Collier, Jan O. Jeppesen, Yi Luo, Julie Perkins, Eric W. M. Wong, James R. Heath, J. Fraser Stoddart
Abstract
Solid-state tunnel junction devices were fabricated from Langmuir Blodgett molecular monolayers of a bistable [2]catenane, a bistable [2]pseudorotaxane, and a single-station [2]rotaxane. All devices exhibited a (noncapacitive) hysteretic current-voltage response that switched the device between high- and low-conductivity states, although control devices exhibited no such response. Correlations between the structure and solution-phase dynamics of the molecular and supramolecular systems, the crystallographic domain structure of the monolayer film, and the room-temperature device performance characteristics are reported.
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