Lasonolide A: Structural Revision and Synthesis of the Unnatural (−)-Enantiomer
Journal of the American Chemical Society2001Vol. 124(3), pp. 384–385
Citations Over TimeTop 10% of 2001 papers
Abstract
Total synthesis of the unnatural (-)-enantiomer of lasonolide A was achieved starting from ethyl l-malate. The two tetrahydropyranyl fragments were prepared stereoselectively via radical cyclization reactions of beta-alkoxyacrylates. The full structure of natural lasonolide A was determined unequivocally.
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