Supramolecular Assembly on Surfaces: Manipulating Conductance in Noncovalently Modified Mesoscale Structures
Journal of the American Chemical Society2002Vol. 124(31), pp. 9036–9037
Citations Over TimeTop 10% of 2002 papers
Grace M. Credo, Andrew K. Boal, Kanad Das, Trent H. Galow, Vincent M. Rotello, Daniel L. Feldheim, Christopher B. Gorman
Abstract
Molecules capable of complementary hydrogen bonding were used to control the noncovalent self-assembly and electronic properties of a chemically well-defined surface mesostructure. In this work, we patterned a footprint region for molecular assembly on a surface and used moieties featuring complementary recognition to tune the current-voltage properties of the patterned region. With the appropriate functionalities on the complementary moieties, we were able to increase and decrease the observed conductance in surface-bound mesoscale structures imaged by scanning tunneling microscopy (STM).
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