Reduction of N2 to Ammonia and Hydrazine Utilizing H2 as the Reductant
Journal of the American Chemical Society2005Vol. 127(29), pp. 10184–10185
Citations Over TimeTop 10% of 2005 papers
Abstract
The trans-Fe(DMeOPrPE)2Cl2 complex (where DMeOPrPE = 1,2-bis(bis(methoxypropyl)phosphino)ethane) undergoes a series of reactions that involve the activation of both H2 and N2 to produce ammonia and hydrazine. A Leigh-type cycle was employed to achieve laboratory fixation of dinitrogen at room temperature and pressure utilizing H2 as the reductant.
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