Time-Dependent Photoluminescence Blue Shift of the Quantum Dots in Living Cells: Effect of Oxidation by Singlet Oxygen
Journal of the American Chemical Society2006Vol. 128(41), pp. 13396–13401
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Yù Zhang, Jiaqi He, Pei-Nan Wang, Ji-Yao Chen, Zhou-Jun Lu, Daru Lu, Jia Guo, Changchun Wang, Wuli Yang
Abstract
Time-dependent photoluminescence (PL) enhancement, blue shift, and photobleach were observed from the thiol-capped CdTe quantum dots (QDs) ingested in mouse myoblast cells and human primary liver cancer cells. It was revealed that the PL blue shift resulted from the photooxidation of the QD core by singlet oxygen molecules formed on the QD core surface.
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