Bifunctional [c2]Daisy-Chains and Their Incorporation into Mechanically Interlocked Polymers
Journal of the American Chemical Society2007Vol. 129(29), pp. 8944–8945
Citations Over TimeTop 10% of 2007 papers
Abstract
A strategy for the formation of mechanically interlocked polymers is presented. Ring-closing olefin metathesis has been shown to provide a very high yielding route to [c2]daisy-chains suitably functionalized to allow their one-step conversion to bisolefins which can be used as monomers in ADMET polymerizations to afford mechanically interlocked polymers. Metathesis, in two different guises is making a hitherto unreachable goal in synthesis a reality.
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