A Chiral Ferromagnetic Molecular Metal
Journal of the American Chemical Society2010Vol. 132(27), pp. 9271–9273
Citations Over TimeTop 10% of 2010 papers
José Ramón Galán‐Mascarós, Eugenio Coronado, Paul Goddard, John Singleton, A. I. Coldea, John D. Wallis, Simon J. Coles, Antonio Alberola
Abstract
The first molecular material with the coexistence of ferromagnetism, metal-like conductivity, and chirality has been prepared using an organic/inorganic approach. In this case, a two-dimensional packing of chiral organic radical cations (responsible for both the electrical conductivity and optical activity) was assembled with a layered bimetallic oxalate-based anionic network (responsible for the magnetic properties). Shubnikov-de Haas oscillations confirmed the presence of a Fermi surface even when the transport properties suggested "insulating"-type behavior at very low temperatures.
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