Direct Arylation of Polycyclic Aromatic Hydrocarbons through Palladium Catalysis
Journal of the American Chemical Society2011Vol. 133(28), pp. 10716–10719
Citations Over TimeTop 10% of 2011 papers
Abstract
We have discovered that the combination of Pd(OAc)(2)/o-chloranil can catalyze the direct C-H bond arylation of polycyclic aromatic hydrocarbons (PAHs) with arylboroxins that occurs selectively at the K-region. The sequential integration of Pd-catalyzed direct arylation of PAHs and FeCl(3)-mediated cyclodehydrogenation is effective in rapidly extending a parent PAH π-system with high directionality.
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