Cooperatively Assembling Donor–Acceptor Superstructures Direct Energy Into an Emergent Charge Separated State
Journal of the American Chemical Society2014Vol. 136(22), pp. 7809–7812
Citations Over TimeTop 10% of 2014 papers
Abstract
A novel supramolecular system composed of diketopyrrolopyrrole electron donors and perylene derived bisimide (PDI) electron acceptors forms superstructures that undergo fast photoinduced charge separation following assembly. This bioinspired route toward functional hierarchical structures, whereby assembly and electronic properties are closely coupled, could lead to new materials for artificial photosynthesis and organic electronics.
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