Low Temperature CO Oxidation over Supported Ultrathin MgO Films
Journal of the American Chemical Society2009Vol. 131(46), pp. 16636–16637
Citations Over TimeTop 10% of 2009 papers
Abstract
Density functional theory is used to investigate CO oxidation over an ultrathin MgO film supported on Ag(100). O(2) is found to be activated on MgO/Ag(100) whereas CO is only weakly bonded to the surface. These adsorption properties together with a low activation barrier render the MgO/Ag system an efficient catalyst for CO oxidation at low temperatures. As the predicted mechanism is general in nature, the result is suggested to have implications for a wide range of oxidation reactions.
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