Catalytic Activity of the Rh Surface Oxide: CO Oxidation over Rh(111) under Realistic Conditions
The Journal of Physical Chemistry C2010Vol. 114(10), pp. 4580–4583
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Johan Gustafson, Rasmus Westerström, Olivier Balmès, Andrea Resta, Richard M. van Rijn, X. Torrelles, C. T. Herbschleb, J.W.M. Frenken, Edvin Lundgren
Abstract
Using a combination of surface X-ray diffraction and mass spectrometry at realistic pressures, the CO oxidation reactivity of a Rh(111) model catalyst has been studied in conjunction with the surface structure. The measurements show that a specific thin surface oxide is always present in the high activity regime of Rh-based CO oxidation.
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