Heterogeneous Reactions in Liquid Sulfuric Acid: HOCl + HCl as a Model System
The Journal of Physical Chemistry1996Vol. 100(16), pp. 6397–6405
Citations Over TimeTop 10% of 1996 papers
Abstract
We describe detailed studies of the interaction of HCl and HOCl with 60 wt % liquid sulfuric acid at 251−276 K as an example of research aimed at understanding the heterogeneous chemistry of the stratosphere. The theory of gas/particle kinetics coupled with measurements of the uptake of HCl and HOCl by bulk and particulate 60 wt % sulfuric acid yield the solubilities of HCl and HOCl, the HCl and HOCl mass accommodation coefficients, the HCl + HOCl liquid-phase rate coefficient, and the HOCl liquid-phase diffusion coefficient. These results are in very good agreement with theoretical predictions and extrapolations of other independent results.
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