Mutational Analysis of the Enterocin Favorskii Biosynthetic Rearrangement
Organic Letters2002Vol. 4(6), pp. 957–960
Citations Over TimeTop 10% of 2002 papers
Abstract
[reaction: see text] A mutational analysis of the enterocin biosynthesis genes revealed that the putative oxygenase and the methyltransferase gene products EncM and EncK, respectively, jointly catalyze a biosynthetic Favorskii-like rearrangement. Inactivation of either gene terminated enterocin production and caused the accumulation of four nonrearranged, nonmethylated polyketides. The structure elucidation of the new wailupemycins E-G is reported.
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