Silver(I) Mediated Folding of a Molecular Basket
Organic Letters2007Vol. 9(12), pp. 2301–2304
Citations Over TimeTop 17% of 2007 papers
Zhiqing Yan, Shijing Xia, M. Gardlik, Wanji Seo, Veselin Maslak, Judith C. Gallucci, Christopher M. Hadad, Jovica D. Badjić
Abstract
We have investigated Ag(I) mediated folding of a tridentate compound, containing three pyridine flaps tethered to a semirigid scaffold, into a molecular basket, using both experimental and theoretical methods. The basket formation has been shown to be highly favorable in organic media (Delta G degrees = -7.2 kcal/mol), with the assembly process allowing for another ligand to bind preferentially on the outer side.
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