Palladium-Catalyzed One-Pot Diarylamine Formation from Nitroarenes and Cyclohexanones
Organic Letters2012Vol. 14(7), pp. 1692–1695
Citations Over TimeTop 10% of 2012 papers
Abstract
The first palladium-catalyzed diarylamine formation from nitroarenes and cyclohexanone derivatives using borrowed hydrogen is described. Various diarylamines were selectively obtained in good to excellent yields. The reaction tolerated a wide range of functionalities. The nitro reduction, cyclohexanone dehydrogenation, and imine formation and reduction were realized in a cascade without an external reducing reagent and oxidant.
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