Divergent Total Synthesis of Taiwaniaquinones A and F and Taiwaniaquinols B and D
Organic Letters2013Vol. 15(8), pp. 2022–2025
Citations Over TimeTop 10% of 2013 papers
Abstract
A divergent approach was developed toward the total synthesis of taiwaniaquinoids. An advanced intermediate 5a with trans A/B ring junction was concisely assembled by employing a Bi(OTf)3-catalyzed cationic cyclization and a Wolff-type ring contraction as key steps. This common intermediate was readily converted to racemic taiwaniaquinones A and F and taiwaniaquinols B and D, respectively.
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