Total Synthesis of Gambierol
Organic Letters2009Vol. 11(19), pp. 4382–4385
Citations Over TimeTop 10% of 2009 papers
Abstract
The total synthesis of gambierol has been achieved utilizing an oxiranyl anion strategy in an iterative manner. Synthetic highlights of this route include direct carbon-carbon formation on epoxides, sulfonyl-assisted 6-endo cyclization, and expansion reaction of tetrahydropyranyl rings to oxepanes to forge the polycyclic architecture of the target molecule.
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