Luminescent cyclometallated Ir(iii) and Pt(ii) complexes with β-diketonate ligands as highly active second-order NLO chromophores
Chemical Communications2010Vol. 46(14), pp. 2414–2414
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Adriana Valore, Alessia Colombo, Claudia Dragonetti, Stefania Righetto, Dominique Roberto, Renato Ugo, Filippo De Angelis, Simona Fantacci
Abstract
[Ir(ppy)(2)(RCOCR'COR)] and [Pt(ppy)(RCOCHCOR)] (ppy = cyclometallated 2-phenylpyridine; R = Me, Ph; R' = H, 2,4-dinitrophenyl) complexes show an unexpected large second order non linear optical response, as evidenced by the EFISH technique, which can be attributed by an SOS-TDDFT investigation mainly to intraligand charge transfer transitions involving the cyclometallated ligands.
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