Exogenous-oxidant-free electrochemical oxidative C–H sulfonylation of arenes/heteroarenes with hydrogen evolution
Chemical Communications2018Vol. 54(81), pp. 11471–11474
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Yong Yuan, Yi Yu, Jin Li Qiao, Pan Liu, Banying Yu, Wukun Zhang, Huilin Liu, Min He, Zhiliang Huang, Aiwen Lei
Abstract
An efficient and environmentally benign electrochemical oxidative radical C-H sulfonylation of arenes/heteroarenes was developed in this work. A series of significant diarylsulfones were prepared under mild catalyst- and exogenous-oxidant-free reaction conditions, which efficiently avoid the issues of desulfonylation or over-reduction of sulfonyl groups.
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