The golden goal of entatic state model design: lowering the internal reorganization energy leads to exponential increase in electron transfer rate
Chemical Communications2025Vol. 61(18), pp. 3684–3687
Citations Over TimeTop 25% of 2025 papers
Abstract
We report a novel guanidine quinolinyl entatic state model system with an electron transfer rate on the order of 105 M-1 s-1 and remarkably little internal reorganization. Comparison between this system and previously reported TMGqu systems reveals an exponential correlation between the internal reorganization energy and the electron transfer rate.
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