Spectral variation of fixed-molecule photoelectron angular distributions
The Journal of Chemical Physics1976Vol. 65(8), pp. 3158–3160
Citations Over TimeTop 10% of 1976 papers
Abstract
We have computed the angular distribution of electrons ejected by electric-dipole interaction from the K shells of CO and N2 molecules held fixed in space, e.g., by adsorption onto a surface. The predicted distributions are very rich in structure, manifesting directly the spectral variation of the orbital momentum composition of the photocurrent. Experimental determination of such distributions will provide a sensitive, detailed probe of molecular photoionization dynamics.
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