Abnormal anti-Stokes Raman scattering of carbon nanotubes
Physical review. B, Condensed matter2002Vol. 66(3)
Citations Over TimeTop 23% of 2002 papers
Shulin Zhang, Xinhua Hu, Hongdong Li, Zujin Shi, Kwok To Yue, Jian Zi, Zhennan Gu, Xiaohua Wu, Zilong Lian, Yong Zhan, Fumin Huang, Lixia Zhou, Yuegang Zhang, Sumio Iijima
Abstract
Abnormal anti-Stokes Raman scattering (AASR) was unambiguously observed in carbon nanotubes (CNT's). In contrast to traditional Raman scattering theory, the absolute value of the Raman frequency of the anti-Stokes peak is not the same as that of the corresponding Stokes peak. It was demonstrated that AASR scattering originates from the unique nanoscale cylindrical structure of CNT's that can be considered naturally as a graphite structure with an intrinsic defect from its rolling. The double-resonance Raman scattering theory was applied to interpret the scattering mechanism of the AASR phenomenon successfully and quantitatively.
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