Coherent molecular vibrational motion observed in the time domain through impulsive stimulated Raman scattering
IEEE Journal of Quantum Electronics1988Vol. 24(2), pp. 460–469
Citations Over TimeTop 1% of 1988 papers
Abstract
Femtosecond time-resolved observations of coherent molecular vibrations are carried out through impulse-stimulated Raman scattering (ISRS). Individual cycles of vibrational oscillation, as well as vibrational dephasing, are time resolved. ISRS therefore provides a means through which time-resolved spectroscopy of vibrationally distorted molecules can be carried out. Several experimental configurations involving either crossed excitation pulses or a single excitation pulse are discussed theoretically and demonstrated experimentally.>
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